Scintillating properties of Cs${_2}$ZrCl${_6}$ crystals in the temperature range of 5-300 K

F. Cappella, P. C. F. Di Stefano, E. Ellingwood, J. Hucker, T. Leroy, S. S. Nagorny, V. V. Nahorna, L. Pagnanini, P. Skensved, N. Swidinsky, P. Wang

公開日: 2025/9/30

Abstract

A new comprehensive study on the Cs${_2}$ZrCl${_6}$ (CZC) crystal scintillating properties under different types of irradiation was performed over a wide temperature range from 5 to 300 K. The light yield (LY) at room temperature (RT), measured under irradiation by 662 keV $\gamma$ quanta of $^{137}$Cs, was evaluated to be 53,300$\pm$4,700 photons/MeV corresponding to approximately 71% of its estimated absolute value. The maximum light emission was observed in the temperature interval 135-165 K, where the LY reached 56,900 photons/MeV and 19,700 photons/MeV for $\gamma$ quanta and $\alpha$ particles, respectively. The quenching factor (QF) for $\alpha$ particles increases smoothly from QF = 0.30 at RT to QF = 0.36 at 135 K. The shape of scintillation pulses induced by $\alpha$ particles is characterized by three time-constants (0.3, 2.5 and 11.8 $\mu$s at RT), whereas the average pulse of $\gamma$ induced events is characterized by two time-constants (1.3 and 11.5 $\mu$s at RT). At the same time, scintillating properties and pulse-shape discrimination capability of the CZC exhibit an acute deterioration at temperatures below 135 K. The optimal operating conditions to maximize the scintillating performance of undoped CZC crystals are discussed.

Scintillating properties of Cs${_2}$ZrCl${_6}$ crystals in the temperature range of 5-300 K | SummarXiv | SummarXiv