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Abstract

The electrical control of pure spin current remains a central challenge in spintronics, particularly in time-reversal symmetric systems composed of nonmagnetic elements, where spin and electric fields interact only indirectly. In this work, we develop a theoretical framework for electrically tuning pure spin photocurrent in two-dimensional materials with time-reversal symmetry via a gate electric field. Through theoretical analysis, we demonstrate that in systems with spin-orbit coupling and in-plane mirror symmetry, an out-of-plane electric field induces spin splitting and reversal in the band structure near the Fermi energy, enabling magnitude control and direction reversal of the pure spin photocurrent. To validate this mechanism, we perform first-principles calculations on germanene, an experimentally realized two-dimensional material. Beyond amplitude modulation, we reveal that reversing the direction of the applied electric field leads to a corresponding reversal of the pure spin photocurrent. Furthermore, we show that the pure spin photocurrent can be tuned by varying the photon energy and the incident angle of light, providing additional degrees of control over spin transport. These findings establish a robust strategy for electric-field-controlled pure spin transport in two-dimensional materials, offering new possibilities for the development of optospintronic devices.