📝 SummarXiv

Abstract

The all-electric realization of high spin polarization and efficient charge-to-spin remains a fundamental challenge in spintronics. We report a spin-axis dynamic locking (SADL) effect in altermagnets that enables fully spin-polarized axial currents: an inplane electric field along one axis drives a pure spin-up current, whereas along the orthogonal axis, it generates a pure spin-down current. Notably, a diagonal field produces a pure transverse spin current with 100% charge-to-spin conversion efficiency. This originates from extremely anisotropic sublattice hopping in a 2D altermagnetic lattice, forming a "tent state" with flat bands and orthogonal Fermi contours. Our firstprinciples calculations demonstrate SADL in a broad class of altermagnetic semiconductors (e.g., 2D Cr2WSe4 monolayer and synthesized 3D (BaF)2Mn2Se2O crystal). These materials provide ideal platforms for gate-tunable, all-electrical spintronics, enabling reconfigurable devices whose spin state is controlled solely by the orientation of an applied electric field.