Fate of Topological Dirac Magnons in van der Waals Ferromagnets at Finite Temperature

Rintaro Eto, Ignacio Salgado-Linares, Masahito Mochizuki, Johannes Knolle, Alexander Mook

公開日: 2025/9/17

Abstract

Dirac magnons, the bosonic counterparts of Dirac fermions in graphene, provide a unique platform to explore symmetry-protected band crossings and quantum geometry in magnetic insulators, while promising high-velocity, low-dissipation spin transport for next-generation magnonic technologies. However, their stability under realistic, finite-temperature conditions remains an open question. Here, we develop a comprehensive microscopic theory of thermal magnon-magnon interactions in van der Waals honeycomb ferromagnets, focusing on both gapless and gapped Dirac magnons. Using nonlinear spin-wave theory with magnon self-energy corrections and a T-matrix resummation that captures two-magnon bound states, we quantitatively reproduce temperature- and momentum-dependent energy shifts and linewidths observed experimentally in the gapless Dirac magnon material CrBr$_3$, even near the Curie temperature. Our approach resolves discrepancies between prior theoretical predictions and experiment and highlight the significant role of bound states in enhancing magnon damping at low temperatures. For gapped Dirac magnon materials such as CrI$_3$, CrSiTe$_3$, and CrGeTe$_3$, we find a thermally induced reduction of the topological magnon gap but no evidence of thermally driven topological transitions. Classical atomistic spin dynamics simulations corroborate the gap' s robustness up to the Curie temperature. Furthermore, we establish a practical criterion for observing topological gaps by determining the minimum ratio of Dzyaloshinskii-Moriya interaction to Heisenberg exchange required to overcome thermal broadening throughout the ordered phase, typically around 5%. Our results clarify the interplay of thermal many-body effects and topology in low-dimensional magnets and provide a reliable framework for interpreting spectroscopic experiments.

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