Intersubband polariton -- LO phonon interaction in mid-infrared non-dispersive cavities: experimental demonstration of spontaneous scattering and perspectives towards polariton lasing
Paul Goulain, Mathieu Jeannin, Stefano Pirotta, Adel Bousseksou, Giorgio Biasiol, Iacopo Carusotto, Raffaele Colombelli, Jean-Michel Manceau
公開日: 2025/9/17
Abstract
We report experimental evidence of the interaction between intersubband polaritons and longitudinal optical phonons in non-dispersive mid-infrared cavities, under resonant optical injection. The light emission originating from spontaneous polariton-phonon scattering is observed at a frequency corresponding to an energy shift of one phonon below the pump frequency. Given the extremely low spontaneous scattering rate, we employ a custom-developed quantum mechanical model to numerically demonstrate the feasibility to stimulate such process using a pump-probe scheme. Based on this analysis, we identify a set of experimental conditions under which optical gain may be realized in a mid-infrared intersubband polaritonic system.