Thermal assisted transport of biexcitons in monolayer WSe2
Dorian Béret, Louka Hemmen, Vishwas Jindal, Sreyan Raha, Thierry Amand, Delphine Lagarde, Andrea Balocchi, Cédric Robert, Helene Carrere, Xavier Marie, Pierre Renucci, Laurent Lombez
Published: 2025/10/3
Abstract
Studies of excitonic transport in transition metal dichalcogenide monolayers have attracted increasing interest in recent years in order to develop nano-optoelectronic devices made with 2D materials. These studies began with low to moderate optical excitation regimes, and more recently have focused on high injection regimes where nonlinear effects appear. This article is focused on the transport of biexcitons by spatially and temporally resolved photoluminescence spectroscopy at high excitation flux. The study is carried out on a high-quality WSe$_2$ monolayer encapsulated in hexagonal boron nitride. The results show that a Seebeck current affects transport in connection with the presence of hot biexcitons. In particular, we observe the formation of spatial rings, also called halos, which have been observed in other excitonic gases. These results tend to generalize the importance of high-energy populations in excitonic transport in TMD, even for complex and heavy excitonic particles.