Identification of soft modes in amorphous Al$_{2}$O$_{3}$ via first-principles
Alexander C. Tyner, Joshuah T. Heath, Thue Christian Thann, Vincent P. Michal, Peter Krogstrup, Mark Kamper Svendsen, Alexander V. Balatsky
Published: 2025/2/20
Abstract
Amorphous Al$_{2}$O$_{3}$ is a fundamental component of modern superconducting qubits. While amphorphous oxides offer distinct advantages, such as directional isotropy and a consistent bulk electronic gap, in realistic systems these compounds support two-level systems (TLSs) which couple to the qubit, expediting decoherence. In this work, we perform a first-principles study of amorphous Al$_{2}$O$_{3}$ and identify low-energy modes in the electronic and phonon spectra as a possible origin for TLSs.